Happy new year! Wish you all the best this year.
In conclusion,
When this TPS563231 chip is enabled, it seems to use a lot of currents.
So it doesn't work safely as the voltage drop occurs.
The picture below shows the VIN and Enable signals taken with the scope. There's a 1.2v drop.
The VIN was raised to 5.5V to maintain more than 4.5V even if the voltage dropped, but it is still unstable.
Can you review it?