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TPS61021A: LED driver circuit

Part Number: TPS61021A

I'm looking to use TPS61021A in a LED driver circuit powered by a AAA battery and wanted to model the setup for optimization. The model that I developed gives me results that are inconsistent with the actual circuit. I downloaded the Spice model for the LED from the manufacturer and got the TPS61021A model from a TI representative.

Any tips, or is there an example Pspice setup that I could reference for something like this?

Model:

 

Actual measured values: