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TPS563201: how to define the maximum value of the output current in this buck circuit

Part Number: TPS563201

Hi,

May I ask about how to define the maximum value of the output current in this buck circuit? When I set the output current value beyond the maximum value, the output voltage fall, how can this happen? 

If I raise the input voltage, can the output current be raised too?

I wish to get this reply. Thanks!