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Finding Register of where LED's reside

Hi,

How does one find the registers that are needed to be written to, to set the LED's to on and off.  I found an example in encodedecode, that connects to the I2C bus for retrieving of the IR commands.  And I dont know where to find how they figure out to write 0x17 for IR_HIGH and 0x18 for IR_LOW.  My guess is to write to a LED you will need some register or address to place this into.  I looked at the MSP430 Datasheet thinking there will be something in there, but I couldnt find anything for tihs.

Thanks in advance.