I use the TAS5631 with a TAS3308 Audio Processor, which Modulation Limit is 69.1% default (programmable) and will set it to 97.7% (limit of the TAS5631).
Section “14.12 PWM Channel Delay, Modulation limit and Offset (0x1A)” describes the bits to be set are BS0..BS2 but I can’t find a table which describes which setting is which limit…