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Not at this time, without doing some of the work yourself.
TICS Pro can export the hex register contents in a standard format, which could be used as an input to a program that calls the FTD2XX dll to send the appropriate bytes to the MPSSE on the FT4232. You would need to parse the text file to extract the raw SPI data to send, format it for the relevant MPSSE function, and call the DLL functions yourself. TICS Pro does not support communicating with FT4232 directly at this time.
The capability is planned, eventually, but the expected timeline for this feature is 2025+.
